Teppala, Dharma Teja ; Bernauer, Jan ; Rashid, Aasir ; Pejic, Milan ; Zagorac, Dejan ; Matovic, Branko ; Ionescu, Emanuel (2024)
Single‐Source Precursor Synthesis of a Compositionally Complex Early Transitional Metal Carbonitride (Ti,Zr,Hf,Nb,Ta)NₓC₁₋ₓ.
In: Advanced Engineering Materials, 2024, 26 (18)
doi: 10.26083/tuprints-00028294
Article, Secondary publication, Publisher's Version
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| Item Type: | Article |
|---|---|
| Type of entry: | Secondary publication |
| Title: | Single‐Source Precursor Synthesis of a Compositionally Complex Early Transitional Metal Carbonitride (Ti,Zr,Hf,Nb,Ta)NₓC₁₋ₓ |
| Language: | English |
| Date: | 5 November 2024 |
| Place of Publication: | Darmstadt |
| Year of primary publication: | September 2024 |
| Place of primary publication: | Weinheim |
| Publisher: | Wiley-VCH |
| Journal or Publication Title: | Advanced Engineering Materials |
| Volume of the journal: | 26 |
| Issue Number: | 18 |
| Collation: | 10 Seiten |
| DOI: | 10.26083/tuprints-00028294 |
| Corresponding Links: | |
| Origin: | Secondary publication DeepGreen |
| Abstract: | Compositionally complex transitional metal nitrides are possible candidates for ultra‐high temperature usage and are known for their superior properties due to the high configuration entropy. It is often difficult to synthesize pure metal nitrides in bulk, due to significant oxygen contamination; hence, they are synthesized mainly as thin films through magnetron sputtering, chemical vapor deposition or surface nitridation of high entropy alloys. The present article reports on a single‐phase compositionally complex ceramic, i.e., (Ti₀.₂Zr₀.₂Hf₀.₂Nb₀.₂Ta₀.₂)NₓC₁₋ₓ, that is synthesized for the first time by employing an organometallic precursor route and using a double ammonolysis process. A multidisciplinary approach is performed to study these compositionally complex nitride and carbonitride systems, including experimental and theoretical investigations. |
| Uncontrolled Keywords: | ammonolysis, compositional complexity, DFT, modeling, nitrides |
| Identification Number: | Artikel-ID: 2302165 |
| Status: | Publisher's Version |
| URN: | urn:nbn:de:tuda-tuprints-282946 |
| Additional Information: | Special Issue: Dedicated to Nahum Travitzky |
| Classification DDC: | 500 Science and mathematics > 530 Physics 600 Technology, medicine, applied sciences > 660 Chemical engineering |
| Divisions: | 11 Department of Materials and Earth Sciences > Material Science > Materials and Resources |
| Date Deposited: | 05 Nov 2024 13:13 |
| Last Modified: | 07 Nov 2024 09:07 |
| SWORD Depositor: | Deep Green |
| URI: | https://tuprints.ulb.tu-darmstadt.de/id/eprint/28294 |
| PPN: | 523218524 |
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