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Electrostatic Boundary Conditions and (Electro)chemical Interface Stability

Huang, Binxiang ; Erhart, Paul ; Yang, Tongqing ; Klein, Andreas (2024)
Electrostatic Boundary Conditions and (Electro)chemical Interface Stability.
In: Advanced Materials Interfaces, 2023, 10 (21)
doi: 10.26083/tuprints-00024674
Article, Secondary publication, Publisher's Version

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Item Type: Article
Type of entry: Secondary publication
Title: Electrostatic Boundary Conditions and (Electro)chemical Interface Stability
Language: English
Date: 9 February 2024
Place of Publication: Darmstadt
Year of primary publication: 2023
Place of primary publication: Weinheim
Publisher: Wiley-VCH
Journal or Publication Title: Advanced Materials Interfaces
Volume of the journal: 10
Issue Number: 21
Collation: 6 Seiten
DOI: 10.26083/tuprints-00024674
Corresponding Links:
Origin: Secondary publication DeepGreen

Interface stability is a key factor for stable operation of electronic and electrochemical devices. This contribution introduces an approach for the operando analysis of interfaces using photoelectron spectroscopy employing a solid oxide electrochemical cell. The combined chemical and electronic information provided by the experiment reveals that not only chemical but also electrostatic boundary conditions are essential for interface stability. The approach is demonstrated using (anti‐)ferroelectric (Pb,La)(Zr,Sn,Ti)O₃ dielectrics.

Uncontrolled Keywords: anti‐ferroelectrics, electrochemical cells, interface stability, operando, X‐ray photoelectron spectroscopy
Identification Number: Artikel-ID: 2300332
Status: Publisher's Version
URN: urn:nbn:de:tuda-tuprints-246748
Classification DDC: 500 Science and mathematics > 530 Physics
600 Technology, medicine, applied sciences > 660 Chemical engineering
Divisions: 11 Department of Materials and Earth Sciences > Material Science > Electronic Structure of Materials (ESM)
LOEWE > LOEWE-Schwerpunkte > FLAME - Fermi Level Engineering Antiferroelektrischer Materialien für Energiespeicher und Isolatoren
Date Deposited: 09 Feb 2024 14:00
Last Modified: 18 Apr 2024 06:18
SWORD Depositor: Deep Green
URI: https://tuprints.ulb.tu-darmstadt.de/id/eprint/24674
PPN: 517200864
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