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Reaction Kinetics of an Industrial Front‐End Acetylene Hydrogenation Catalyst Using the Advanced TEMKIN Reactor

Hock, Sebastian ; Iser, Leonhard ; Lucas, Martin ; Rose, Marcus (2022):
Reaction Kinetics of an Industrial Front‐End Acetylene Hydrogenation Catalyst Using the Advanced TEMKIN Reactor. (Publisher's Version)
In: Chemie Ingenieur Technik, 94 (11), pp. 1704-1710. Wiley-VCH, e-ISSN 1522-2640,
DOI: 10.26083/tuprints-00022900,
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Item Type: Article
Origin: Secondary publication DeepGreen
Status: Publisher's Version
Title: Reaction Kinetics of an Industrial Front‐End Acetylene Hydrogenation Catalyst Using the Advanced TEMKIN Reactor
Language: English
Abstract:

The front‐end process integration of the selective acetylene hydrogenation provides several advantages over the tail‐end option. But extensive knowledge of the process and reaction kinetics are required. This work combines the ideal conditions of the advanced TEMKIN reactor in a laboratory plant for gradient‐free kinetic analysis of eggshell catalyst under industrially relevant front‐end conditions. With this system an industrial state of the art Pd‐Ag/Al₂O₃ eggshell catalyst is investigated and the temperature dependent data under various feed compositions including information on the formation of C₄‐species are reported.

Journal or Publication Title: Chemie Ingenieur Technik
Volume of the journal: 94
Issue Number: 11
Place of Publication: Darmstadt
Publisher: Wiley-VCH
Uncontrolled Keywords: Acetylene hydrogenation, Catalysis, Front‐end, Reaction engineering, TEMKIN reactor
Classification DDC: 500 Naturwissenschaften und Mathematik > 540 Chemie
600 Technik, Medizin, angewandte Wissenschaften > 660 Technische Chemie
Divisions: 07 Department of Chemistry > Fachgebiet Technische Chemie > Technische Chemie II
Date Deposited: 28 Nov 2022 14:11
Last Modified: 08 Dec 2022 06:44
DOI: 10.26083/tuprints-00022900
Corresponding Links:
URN: urn:nbn:de:tuda-tuprints-229005
SWORD Depositor: Deep Green
URI: https://tuprints.ulb.tu-darmstadt.de/id/eprint/22900
PPN: 502347260
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