Morozovska, Anna Nickolaevna ; Eliseev, Eugene A. ; Karpinsky, Dmitry V. ; Silibin, Maxim V. ; Vasudevan, Rama ; Kalinin, Sergei V. ; Genenko, Yuri A. (2022)
Mesoscopic theory of defect ordering–disordering transitions in thin oxide films.
In: Scientific Reports, 2022, 10
doi: 10.26083/tuprints-00021109
Article, Secondary publication, Publisher's Version
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Item Type: | Article |
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Type of entry: | Secondary publication |
Title: | Mesoscopic theory of defect ordering–disordering transitions in thin oxide films |
Language: | English |
Date: | 14 April 2022 |
Place of Publication: | Darmstadt |
Year of primary publication: | 2022 |
Publisher: | Springer Nature |
Journal or Publication Title: | Scientific Reports |
Volume of the journal: | 10 |
Collation: | 13 Seiten |
DOI: | 10.26083/tuprints-00021109 |
Corresponding Links: | |
Origin: | Secondary publication via sponsored Golden Open Access |
Abstract: | Ordering of mobile defects in functional materials can give rise to fundamentally new phases possessing ferroic and multiferroic functionalities. Here we develop the Landau theory for strain induced ordering of defects (e.g. oxygen vacancies) in thin oxide films, considering both the ordering and wavelength of possible instabilities. Using derived analytical expressions for the energies of various defect-ordered states, we calculated and analyzed phase diagrams dependence on the film-substrate mismatch strain, concentration of defects, and Vegard coefficients. Obtained results open possibilities to create and control superstructures of ordered defects in thin oxide films by selecting the appropriate substrate and defect concentration. |
Status: | Publisher's Version |
URN: | urn:nbn:de:tuda-tuprints-211092 |
Classification DDC: | 600 Technology, medicine, applied sciences > 600 Technology 600 Technology, medicine, applied sciences > 620 Engineering and machine engineering |
Divisions: | 11 Department of Materials and Earth Sciences > Material Science 11 Department of Materials and Earth Sciences > Material Science > Materials Modelling |
Date Deposited: | 14 Apr 2022 12:09 |
Last Modified: | 14 Nov 2023 19:04 |
URI: | https://tuprints.ulb.tu-darmstadt.de/id/eprint/21109 |
PPN: | 49343318X |
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