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Design of a 1 MWth Pilot Plant for Chemical Looping Gasification of Biogenic Residues

Marx, Falko ; Dieringer, Paul ; Ströhle, Jochen ; Epple, Bernd (2022):
Design of a 1 MWth Pilot Plant for Chemical Looping Gasification of Biogenic Residues. (Publisher's Version)
In: Energies, 14 (9), MDPI, e-ISSN 1996-1073,
DOI: 10.26083/tuprints-00019522,

Copyright Information: CC BY 4.0 International - Creative Commons, Attribution.

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Item Type: Article
Origin: Secondary publication DeepGreen
Status: Publisher's Version
Title: Design of a 1 MWth Pilot Plant for Chemical Looping Gasification of Biogenic Residues
Language: English

Chemical looping gasification (CLG) is a promising process for the thermochemical solid to liquid conversion route using lattice oxygen, provided by a solid oxygen carrier material, to produce a nitrogen free synthesis gas. Recent advances in lab-scale experiments show that CLG with biomass has the possibility to produce a carbon neutral synthesis gas. However, all experiments have been conducted in externally heated units, not enabling autothermal operation. In this study, the modification of an existing pilot plant for demonstrating autothermal operation of CLG is described. Energy and mass balances are calculated using a validated chemical looping combustion process model extended for biomass gasification. Based on six operational cases, adaptations of the pilot plant are designed and changes discussed. A reactor configuration using two circulating fluidized bed reactors with internal solid circulation in the air reactor is proposed and a suitable operating strategy devised. The resulting experimental unit enables a reasonable range of operational parameters within restrictions imposed from autothermal operation.

Journal or Publication Title: Energies
Volume of the journal: 14
Issue Number: 9
Place of Publication: Darmstadt
Publisher: MDPI
Collation: 25 Seiten
Uncontrolled Keywords: chemical looping, biomass, gasification, fluidized bed, autothermal, pilot plant
Classification DDC: 600 Technik, Medizin, angewandte Wissenschaften > 600 Technik
Divisions: 16 Department of Mechanical Engineering > Institut für Energiesysteme und Energietechnik (EST)
Date Deposited: 31 Jan 2022 13:05
Last Modified: 23 Aug 2022 06:47
DOI: 10.26083/tuprints-00019522
Corresponding Links:
URN: urn:nbn:de:tuda-tuprints-195223
SWORD Depositor: Deep Green
URI: https://tuprints.ulb.tu-darmstadt.de/id/eprint/19522
PPN: 492946639
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