Vasala, Sami ; Jakob, Anna ; Wissel, Kerstin ; Waidha, Aamir Iqbal ; Alff, Lambert ; Clemens, Oliver (2024)
Reversible Tuning of Magnetization in a Ferromagnetic Ruddlesden–Popper‐Type Manganite by Electrochemical Fluoride‐Ion Intercalation.
In: Advanced Electronic Materials, 2020, 6 (2)
doi: 10.26083/tuprints-00017042
Article, Secondary publication, Publisher's Version
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| Item Type: | Article |
|---|---|
| Type of entry: | Secondary publication |
| Title: | Reversible Tuning of Magnetization in a Ferromagnetic Ruddlesden–Popper‐Type Manganite by Electrochemical Fluoride‐Ion Intercalation |
| Language: | English |
| Date: | 5 January 2024 |
| Place of Publication: | Darmstadt |
| Year of primary publication: | 2020 |
| Place of primary publication: | Weinheim |
| Publisher: | Wiley-VCH |
| Journal or Publication Title: | Advanced Electronic Materials |
| Volume of the journal: | 6 |
| Issue Number: | 2 |
| Collation: | 9 Seiten |
| DOI: | 10.26083/tuprints-00017042 |
| Corresponding Links: | |
| Origin: | Secondary publication DeepGreen |
| Abstract: | Electrical tuning of materials' magnetic properties is of great technological interest, and in particular reversible on/off switching of ferromagnetism can enable various new applications. Reversible magnetization tuning in the ferromagnetic Ruddlesden–Popper manganite La₂₋₂ₓSr₁₊₂ₓMn₂O₇ by electrochemical fluoride‐ion (de)intercalation in an all‐solid‐state system is demonstrated for the first time. A 67% change in relative magnetization is observed with a low operating potential of <1 V, negligible capacity fading, and high Coulombic efficiency. This system offers a high magnetoelectric voltage coefficient, indicating high energy efficiency. This method can also be extended to tune other materials' properties in various perovskite‐related materials. |
| Uncontrolled Keywords: | fluoride‐ion batteries, magnetoelectrics, manganites, Ruddlesden–Popper perovskites, tunable ferromagnetism |
| Status: | Publisher's Version |
| URN: | urn:nbn:de:tuda-tuprints-170428 |
| Classification DDC: | 600 Technology, medicine, applied sciences > 621.3 Electrical engineering, electronics 600 Technology, medicine, applied sciences > 660 Chemical engineering |
| Divisions: | 11 Department of Materials and Earth Sciences > Material Science > Advanced Thin Film Technology 11 Department of Materials and Earth Sciences > Material Science > Fachgebiet Materialdesign durch Synthese |
| Date Deposited: | 05 Jan 2024 14:14 |
| Last Modified: | 09 Jan 2024 09:29 |
| SWORD Depositor: | Deep Green |
| URI: | https://tuprints.ulb.tu-darmstadt.de/id/eprint/17042 |
| PPN: | 514523093 |
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