Hess, Ch. ; Wolf, M. ; Bonn, M. (2024)
Direct Observation of Vibrational Energy Delocalization on Surfaces: CO on Ru(001).
In: Physical Review Letters, 2000, 85 (20)
doi: 10.26083/tuprints-00026902
Article, Secondary publication, Publisher's Version
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| Item Type: | Article |
|---|---|
| Type of entry: | Secondary publication |
| Title: | Direct Observation of Vibrational Energy Delocalization on Surfaces: CO on Ru(001) |
| Language: | English |
| Date: | 23 April 2024 |
| Place of Publication: | Darmstadt |
| Year of primary publication: | 2000 |
| Place of primary publication: | College Park, MD |
| Publisher: | American Physical Society |
| Journal or Publication Title: | Physical Review Letters |
| Volume of the journal: | 85 |
| Issue Number: | 20 |
| DOI: | 10.26083/tuprints-00026902 |
| Corresponding Links: | |
| Origin: | Secondary publication service |
| Abstract: | We report the experimental observation of the gradual transition from a local oscillator to a two-dimensional delocalized phonon, observed for the CO-stretch vibration of carbon monoxide adsorbed on a Ru(001) surface by means of broadband-infrared saturation sum-frequency spectroscopy. The data are theoretically reproduced by an exchange model with residence times of the excitation down to 2.5 ps. |
| Status: | Publisher's Version |
| URN: | urn:nbn:de:tuda-tuprints-269028 |
| Classification DDC: | 500 Science and mathematics > 530 Physics 500 Science and mathematics > 540 Chemistry |
| Date Deposited: | 23 Apr 2024 08:24 |
| Last Modified: | 02 Aug 2024 08:31 |
| URI: | https://tuprints.ulb.tu-darmstadt.de/id/eprint/26902 |
| PPN: | 520273672 |
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