Novel Surface Vibrational Spectroscopy: Infrared-Infrared-Visible Sum-Frequency Generation

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Item Type:	Article
Type of entry:	Secondary publication
Title:	Novel Surface Vibrational Spectroscopy: Infrared-Infrared-Visible Sum-Frequency Generation
Language:	English
Date:	23 April 2024
Place of Publication:	Darmstadt
Year of primary publication:	2001
Place of primary publication:	College Park, MD
Publisher:	American Physical Society
Journal or Publication Title:	Physical Review Letters
Volume of the journal:	86
Issue Number:	8
DOI:	10.26083/tuprints-00026901
Corresponding Links:	Publisher-DOI
Origin:	Secondary publication service
Abstract:	A novel type of surface vibrational sum-frequency generation spectroscopy is presented that enables a highly specific measurement of the coupling of molecules on surfaces. With this doubly vibrationally resonant technique, two-dimensional vibrational spectroscopy of molecules on surfaces becomes possible. The technique is demonstrated for the C-O stretch vibration of CO on a ruthenium (001) surface. It allows for the determination of the intermolecular coupling strength of dipole-coupled CO molecules on the surface.
Status:	Publisher's Version
URN:	urn:nbn:de:tuda-tuprints-269019
Classification DDC:	500 Science and mathematics > 530 Physics 500 Science and mathematics > 540 Chemistry
Date Deposited:	23 Apr 2024 08:25
Last Modified:	23 Apr 2024 08:25
URI:	https://tuprints.ulb.tu-darmstadt.de/id/eprint/26901
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