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Magnetic flux dynamics and structural features in fluorinated HgBa₂CuO₄ as probed by ¹⁹F NMR

Gippius, Andrei Andreevich ; Morozova, E. N. ; Antipov, Evgeny V. ; Abakumov, Artem M. ; Rozova, M. G. ; Lüders, Klaus ; Hoffmann, W. ; Buntkowsky, Gerd ; Klein, Oliver (2023)
Magnetic flux dynamics and structural features in fluorinated HgBa₂CuO₄ as probed by ¹⁹F NMR.
In: Physical Review B, 2000, 61 (21)
doi: 10.26083/tuprints-00024239
Article, Secondary publication, Publisher's Version

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Item Type: Article
Type of entry: Secondary publication
Title: Magnetic flux dynamics and structural features in fluorinated HgBa₂CuO₄ as probed by ¹⁹F NMR
Language: English
Date: 12 July 2023
Place of Publication: Darmstadt
Year of primary publication: 2000
Publisher: American Physical Society
Journal or Publication Title: Physical Review B
Volume of the journal: 61
Issue Number: 21
DOI: 10.26083/tuprints-00024239
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Origin: Secondary publication service
Abstract:

¹⁹F NMR spectra and spin-lattice relaxation rates have been measured on two powder HgBa₂CuO₄Fₓ samples. The results combined with our neutron powder-diffraction data [A. M. Abakumov et al., Phys. Rev. Lett. 80, 385 (1998)] confirm that fluorine atoms can be successfully incorporated in the lattice of superconducting Hg-1201 phase in the nonstoichiometric O3 site. Partial occupation of another oxygen position by fluorine atoms reveals to be possible with the increase of F content. The temperature dependence of the ¹⁹F NMR linewidth reveals the crossover at 35 K in the magnetic-flux line structure between the low-temperature latticelike regime and high-temperature “melted” regime. For the 1/T₁ temperature dependence a maximum has been found at 65 K indicating the strong influence of magnetic-flux line motion on the ¹⁹F spin-lattice relaxation rate.

Status: Publisher's Version
URN: urn:nbn:de:tuda-tuprints-242393
Classification DDC: 500 Science and mathematics > 530 Physics
500 Science and mathematics > 540 Chemistry
Divisions: 07 Department of Chemistry > Eduard Zintl-Institut > Physical Chemistry
Date Deposited: 12 Jul 2023 12:58
Last Modified: 06 Oct 2023 09:08
URI: https://tuprints.ulb.tu-darmstadt.de/id/eprint/24239
PPN: 512061009
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