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  5. Advancing Radiation-Detected Resonance Ionization towards Heavier Elements and More Exotic Nuclides
 
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2022
Zweitveröffentlichung
Artikel
Verlagsversion

Advancing Radiation-Detected Resonance Ionization towards Heavier Elements and More Exotic Nuclides

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Hauptpublikation
atoms-10-00041-v2.pdf
CC BY 4.0 International
Format: Adobe PDF
Size: 2 MB
TUDa URI
tuda/8669
URN
urn:nbn:de:tuda-tuprints-212806
DOI
10.26083/tuprints-00021280
Autor:innen
Warbinek, Jessica ORCID 0000-0002-2385-5584
Anđelić, Brankica
Block, Michael ORCID 0000-0001-9282-8347
Chhetri, Premaditya
Claessens, Arno
Ferrer, Rafael
Giacoppo, Francesca ORCID 0000-0001-9592-5230
Kaleja, Oliver
Kieck, Tom ORCID 0000-0003-3146-4994
Kim, EunKang
Laatiaoui, Mustapha ORCID 0000-0003-0105-8303
Lantis, Jeremy
Mistry, Andrew
Münzberg, Danny
Nothhelfer, Steven ORCID 0000-0002-8089-1872
Raeder, Sebastian ORCID 0000-0003-0505-1440
Rey-Herme, Emmanuel
Rickert, Elisabeth
Romans, Jekabs ORCID 0000-0001-9742-7745
Romero-Romero, Elisa ORCID 0000-0003-4015-4904
Vandebrouck, Marine
Duppen, Piet van ORCID 0000-0002-5053-7370
Walther, Thomas ORCID 0000-0001-8114-1785
Kurzbeschreibung (Abstract)

RAdiation-Detected Resonance Ionization Spectroscopy (RADRIS) is a versatile method for highly sensitive laser spectroscopy studies of the heaviest actinides. Most of these nuclides need to be produced at accelerator facilities in fusion-evaporation reactions and are studied immediately after their production and separation from the primary beam due to their short half-lives and low production rates of only a few atoms per second or less. Only recently, the first laser spectroscopic investigation of nobelium (Z=102) was performed by applying the RADRIS technique in a buffer-gas-filled stopping cell at the GSI in Darmstadt, Germany. To expand this technique to other nobelium isotopes and for the search for atomic levels in the heaviest actinide element, lawrencium (Z=103), the sensitivity of the RADRIS setup needed to be further improved. Therefore, a new movable double-detector setup was developed, which enhances the overall efficiency by approximately 65% compared to the previously used single-detector setup. Further development work was performed to enable the study of longer-lived (t₁/₂>1 h) and shorter-lived nuclides (t₁/₂<1 s) with the RADRIS method. With a new rotatable multi-detector design, the long-lived isotope 254Fm (t₁/₂=3.2 h) becomes within reach for laser spectroscopy. Upcoming experiments will also tackle the short-lived isotope 251No (t₁/₂=0.8 s) by applying a newly implemented short RADRIS measurement cycle.

Freie Schlagworte

laser spectroscopy

resonance ionization

atomic level scheme

gas cell

radiation detection

heavy actinides

Sprache
Englisch
Fachbereich/-gebiet
05 Fachbereich Physik > Institut für Angewandte Physik
05 Fachbereich Physik > Institut für Kernphysik
DDC
500 Naturwissenschaften und Mathematik > 530 Physik
Institution
Universitäts- und Landesbibliothek Darmstadt
Ort
Darmstadt
Titel der Zeitschrift / Schriftenreihe
Atoms
Jahrgang der Zeitschrift
10
Heftnummer der Zeitschrift
2
ISSN
2218-2004
Verlag
MDPI
Publikationsjahr der Erstveröffentlichung
2022
Verlags-DOI
10.3390/atoms10020041
PPN
499802969

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