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Reaction Kinetics of an Industrial Front‐End Acetylene Hydrogenation Catalyst Using the Advanced TEMKIN Reactor

Hock, Sebastian ; Iser, Leonhard ; Lucas, Martin ; Rose, Marcus (2022)
Reaction Kinetics of an Industrial Front‐End Acetylene Hydrogenation Catalyst Using the Advanced TEMKIN Reactor.
In: Chemie Ingenieur Technik, 2022, 94 (11)
doi: 10.26083/tuprints-00022900
Article, Secondary publication, Publisher's Version

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Item Type: Article
Type of entry: Secondary publication
Title: Reaction Kinetics of an Industrial Front‐End Acetylene Hydrogenation Catalyst Using the Advanced TEMKIN Reactor
Language: English
Date: 28 November 2022
Place of Publication: Darmstadt
Year of primary publication: 2022
Publisher: Wiley-VCH
Journal or Publication Title: Chemie Ingenieur Technik
Volume of the journal: 94
Issue Number: 11
DOI: 10.26083/tuprints-00022900
Corresponding Links:
Origin: Secondary publication DeepGreen
Abstract:

The front‐end process integration of the selective acetylene hydrogenation provides several advantages over the tail‐end option. But extensive knowledge of the process and reaction kinetics are required. This work combines the ideal conditions of the advanced TEMKIN reactor in a laboratory plant for gradient‐free kinetic analysis of eggshell catalyst under industrially relevant front‐end conditions. With this system an industrial state of the art Pd‐Ag/Al₂O₃ eggshell catalyst is investigated and the temperature dependent data under various feed compositions including information on the formation of C₄‐species are reported.

Uncontrolled Keywords: Acetylene hydrogenation, Catalysis, Front‐end, Reaction engineering, TEMKIN reactor
Status: Publisher's Version
URN: urn:nbn:de:tuda-tuprints-229005
Classification DDC: 500 Science and mathematics > 540 Chemistry
600 Technology, medicine, applied sciences > 660 Chemical engineering
Divisions: 07 Department of Chemistry > Ernst-Berl-Institut > Fachgebiet Technische Chemie > Technische Chemie II
Date Deposited: 28 Nov 2022 14:11
Last Modified: 14 Nov 2023 19:05
SWORD Depositor: Deep Green
URI: https://tuprints.ulb.tu-darmstadt.de/id/eprint/22900
PPN: 502347260
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